Journal
ENERGIES
Volume 5, Issue 7, Pages 2449-2498Publisher
MDPI
DOI: 10.3390/en5072449
Keywords
methane; gas hydrate; marine sediments; global change
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Funding
- German ministry for research (BMBF)
- German ministry for economics (BMWI)
- German research foundation (DFG) through Kiel-based Cluster of Excellence The Future Ocean
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The accumulation of methane hydrate in marine sediments is controlled by a number of physical and biogeochemical parameters including the thickness of the gas hydrate stability zone (GHSZ), the solubility of methane in pore fluids, the accumulation of particulate organic carbon at the seafloor, the kinetics of microbial organic matter degradation and methane generation in marine sediments, sediment compaction and the ascent of deep-seated pore fluids and methane gas into the GHSZ. Our present knowledge on these controlling factors is discussed and new estimates of global sediment and methane fluxes are provided applying a transport-reaction model at global scale. The modeling and the data evaluation yield improved and better constrained estimates of the global pore volume within the modern GHSZ (>= 44 x 10(15) m(3)), the Holocene POC accumulation rate at the seabed (similar to 1.4 x 10(14) g yr(-1)), the global rate of microbial methane production in the deep biosphere (4-25 x 10(12) g C yr(-1)) and the inventory of methane hydrates in marine sediments (>= 455 Gt of methane-bound carbon).
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