Journal
ELECTRONIC MATERIALS LETTERS
Volume 8, Issue 2, Pages 199-207Publisher
KOREAN INST METALS MATERIALS
DOI: 10.1007/s13391-012-2038-6
Keywords
solid-state battery; lithium battery; solid electrolyte; glass; glass-ceramic; nanocomposite
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Funding
- Ministry of Education, Culture, Sports, Science and Technology of Japan
- Japan Science and Technology Agency (JST), Core Research for Evolutional Science and Technology (CREST)
- Grants-in-Aid for Scientific Research [21246098] Funding Source: KAKEN
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The recent development of bulk-type solid-state rechargeable lithium batteries with sulfide glass-ceramics as a solid electrolyte was reviewed. Sulfide glasses and glass-ceramics in the system Li2S-P(2)S(5)have an advantage of high conductivity, wide electrochemical window and low grain-boundary resistance. Bulk-type solid-state batteries composed of compressed powder layers of electrode and electrolyte were fabricated with Li2S-P2S5 glass-ceramic electrolytes. Formation of a favorable solid-solid interface between electrode and electrolyte is a key to achieving excellent performance in solid-state batteries. The mechanochemical preparation of nanocomposite electrodes and surface modification of active materials by softening of the electrolyte, or PLD coating, were useful for increasing the electrode-electrolyte contact area and improving battery performance.
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