Journal
ELECTROCHIMICA ACTA
Volume 76, Issue -, Pages 326-332Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.electacta.2012.05.038
Keywords
Nano-Si; Multi-wall carbon nanotube; Sodium carboxymethyl cellulose; Free-standing electrode; Lithium-ion battery
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Funding
- National Science Foundation of China [50973112]
- Hundred Talents Program of Chinese Academy of Sciences (CAS)
- CAS-Guangdong Collaboration Program [20108]
- Guangzhou Municipal Project for Science Technology [11A44061500]
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Nano-Si/(multi-wall carbon nanotube) (Si/MWCNT) composite paper was prepared as flexible electrode for lithium ion batteries by a simple filtration method using sodium carboxymethyl cellulose (CMC) as a dispersing/binding agent, followed by a thermal sintering process. Scanning electron microscopy (SEM) showed that nanosized Si particles were dispersed homogeneously and intertwined by the MWCNT throughout the whole paper electrode. After thermal sintering, Si/MWCNT paper electrode exhibited a significantly improved flexibility with a high Si content of 35.6 wt% as compared with before sintering, and retained a specific capacity of 942 mAh g(-1) after 30 cycles with a capacity fade of 0.46%/cycle. (C) 2012 Elsevier Ltd. All rights reserved.
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