4.6 Review

Recent trends and developments in polymer electrolyte membrane fuel cell modelling

Journal

ELECTROCHIMICA ACTA
Volume 56, Issue 11, Pages 3731-3757

Publisher

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.electacta.2010.10.046

Keywords

PEM fuel cell; Modelling and simulation; Dynamic; Degradation; Multiscale

Funding

  1. EPSRC [EP/E011640/1] Funding Source: UKRI
  2. Engineering and Physical Sciences Research Council [EP/E011640/1] Funding Source: researchfish

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Modelling and simulation are well-established tools for investigating the physical processes inside a polymer electrolyte membrane (PEM) fuel cell. The early literature paid great attention to steady-state transport phenomena in the main components, which continues to be a focus of ongoing activities. There is, on the other hand, a growing interest in modelling other aspects of fuel cell operation, such as transient performance and degradation phenomena. There has also been a growth in the number of molecular and pore-level studies of transport phenomena in fuel cell components, enabled by developments in simulation techniques and enhancements in computer hardware. Such approaches are capable of representing important small-scale phenomena more faithfully than traditional macroscopic models. This review summarises recent activity in PEM fuel cell modelling, with a focus on detailed physical models, and considers its potential significance. An industrial perspective is also provided, highlighting the current use of modelling in the test and design cycles, and outlining future requirements. (C) 2010 Elsevier Ltd. All rights reserved.

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