Journal
ELECTROCHIMICA ACTA
Volume 56, Issue 3, Pages 1037-1042Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.electacta.2010.10.042
Keywords
Electron transfer-induced; Four-membered cyclic intermediate; Radical cation; Olefin cross-coupling; Olefin cross-metathesis
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Funding
- Ministry of Education, Culture, Sports, Science, and Technology
- Grants-in-Aid for Scientific Research [21380072] Funding Source: KAKEN
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An electron transfer-induced four-membered cyclic intermediate, formed between a radical cation of an enol ether and an unactivated olefin. played a key role in the pathway toward either cross-coupling or cross-metathesis. The presence of an alkoxy group on the phenyl ring of the olefin entirely determined the synthetic outcome of the reaction, which mirrored the efficiency of the intramolecular electron transfer. (C) 2010 Elsevier Ltd. All rights reserved.
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