Journal
ELECTROCHEMISTRY COMMUNICATIONS
Volume 10, Issue 11, Pages 1801-1804Publisher
ELSEVIER SCIENCE INC
DOI: 10.1016/j.elecom.2008.09.021
Keywords
gamma-Ray irradiation; High Pt loading; Electrocatalyst; Cathode; Direct methanol fuel cell
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Funding
- Korean Research Foundation [KRF-2008314-C00175]
- BK21 Program
- Korean Basic Science Institute at Jeonju and Deajeon
- National Research Foundation of Korea [2008-314-C00175] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
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In this study, a gamma-ray irradiation approach without addition of any commonly used reducing chemicals has been explored to synthesize carbon-supported high Pt loading (i.e., 80 wt.%) cathode catalyst for direct methanol fuel cell. Compared with the Pt catalyst prepared by impregnation-NaBH4 reduction approach, the supported Pt catalyst synthesized by gamma-ray irradiation has better dispersion of Pt nano-particles on the carbon support with smaller particle size and narrower size distribution and has demonstrated enhanced catalytic activity toward oxygen reduction reaction and improved fuel cell performance. (c) 2008 Elsevier B.V. All rights reserved.
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