Journal
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
Volume 6, Issue 15, Pages 3054-3060Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.jpclett.5b01059
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Funding
- European Research Council [321305]
- Royal Society
- Scottish Doctoral Training Centre [EP/L015110/1]
- EPSRC [EP/J009016]
- Thuringer Landesgraduiertenschule fur Photovoltaik (PhotoGrad)
- Deutsche Forschungsgemeinschaft (DFG) [SPP1355]
- Engineering and Physical Sciences Research Council [EP/J009016/1] Funding Source: researchfish
- EPSRC [EP/J009016/1] Funding Source: UKRI
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The influence of crystallinity on exciton diffusion and fullerene distribution was investigated by blending amorphous and semicrystalline copolymers. We measured exciton diffusion and fluorescence quenching in such blends by dispersing fullerene molecules into them. We find that the diffusion length is more than two times higher in the semicrystalline copolymer than in the amorphous copolymer. We also find that fullerene preferentially mixes into disordered regions of the polymer film. This shows that relatively small differences in molecular structure are important for exciton diffusion and fullerene distribution.
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