Journal
DALTON TRANSACTIONS
Volume 47, Issue 41, Pages 14706-14712Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8dt03161d
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Funding
- National Natural Science Foundation of China [21476097, 21776118]
- Natural Science Foundation of Jiangsu Province [BK20161363]
- China Postdoctoral Science Foundation [2017M620193]
- Key Laboratory of Tropical Medicinal Plant Chemistry of Ministry of Education-Hainan Normal University [rdyw2018002]
- Priority Academic Program Development of Jiangsu Higher Education Institutions
- high performance computing platform of Jiangsu University
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Photocatalysis is a promising technology which can be applied in the fields of energy and environment. However, low charge separation efficiency has limited its commercial applications. In this work, we report a route to a controllable synthesized visible-light-driven heterostructure photocatalyst Mo2C@C/2D g-C3N4. The interfacial conductivity was improved by introducing Mo2C@C, which promoted the transportation of photogenerated carriers and suppressed their recombination. The optimal composite achieved a hydrogen (H-2) generation rate of 2269.47 mu mol g(-1) h(-1), and an external quantum efficiency (EQE) achieved 9.07% at lambda = 405 nm. Thus, the great co-catalytic activity of Mo2C@C was unambiguously
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