Journal
DALTON TRANSACTIONS
Volume 43, Issue 41, Pages 15300-15304Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4dt02264e
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Funding
- Fraunhofer Society [MAVO 824 704]
- University of Dusseldorf
- State of Baden-Wurttemberg for funds of the Baden-Wurttemberg Research Program Securing a Sustainable Living Environment (BWPLUS) [BWE 12001]
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The hydrothermal stability of aluminium hydroxide isophthalate MOF CAU-10-H was proven, under humid multi-cycling conditions. Detailed in situ thermogravimetric measurements and in situ powder X-ray diffraction analysis during water ad-/desorption were used. A reversible structural change during adsorption was detected and thereby exemplified the robustness of breathing-like MOFs over 700 water vapour ad/desorption cycles. In combination with high water adsorption capacity, hydrophilic CAU-10-H is the first breathing-like MOF with a structural change which is a promising candidate for the use in heat transformation processes.
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