Journal
DALTON TRANSACTIONS
Volume 43, Issue 29, Pages 11333-11338Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4dt00827h
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Funding
- National Natural Science Foundation of China [21273192, 61204009]
- Innovation Scientists and Technicians Troop Construction Projects of Henan Province [144200510014]
- Program for Science & Technology Innovation Talents in Universities of Henan Province [2011HASTIT029]
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Silver oxides (Ag2O and AgO) have attracted increasing attention as potential solar cell materials for photovoltaic devices due to their ideal bandgap and non-toxicity. In order to eliminate the complicated synthesis and harsh reaction conditions (e.g. high temperature, high vacuum, high energy input, electron beam instrumentation) required by most synthetic strategies, we developed a very facile dry chemical approach to directly prepare AgxO species on the ITO substrate by taking advantage of a UV-O-3 surrounding in a controlled way. We systematically investigated the effects of relative humidity, reaction temperature, and the silver deposition technique on the formation of silver oxide (AgO or Ag2O) thin films. A possible synthetic mechanism for the formation of AgO and Ag2O is proposed. More importantly, we have designed and successfully fabricated novel inorganic hybrid Ag2O/Bi2O3 heterojunction thin films for the first time which exhibit significantly improved photocurrent compared with pure Bi2O3 films.
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