Journal
DALTON TRANSACTIONS
Volume 41, Issue 23, Pages 7134-7140Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2dt30353a
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- Institute for Advanced Studies in Basic Sciences
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Nano-sized layered aluminium or zinc-manganese oxides were synthesized and characterized by scanning electron microscopy, transmission electron microscopy, X-ray diffraction spectrometry, dynamic light scattering and atomic absorption spectroscopy. These oxides showed efficient water oxidizing activity in the presence of cerium(IV) ammonium nitrate as a non-oxo transfer oxidant. Amounts of dissolved manganese, zinc or aluminium, and water oxidation activities of these oxides were reported and compared with other manganese oxides. A mechanism for oxygen evolution and possible roles for zinc or aluminium ions are also proposed.
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