Journal
CURRENT ORGANIC CHEMISTRY
Volume 13, Issue 9, Pages 919-938Publisher
BENTHAM SCIENCE PUBL LTD
DOI: 10.2174/138527209788452135
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Funding
- Spanish Ministry of Education and Science [CTQ-2005-01834-BQU, CTQ-2007-64843-BQU]
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Intramolecular haloetherification and transannular hydroxycyclization of alkenes is a synthetic methodology to obtain polycyclic ethers and amines in a regio- and stereoselective manner. The stereoelectronic effects controlling this selectivity are discussed. Also, the methodology based on [4+3]-cycloaddition followed by intramolecular haloetherification or transannular hydroxycyclization is described as a very useful tool to prepare the dioxa- and oxazatricyclic cores of several bioactive natural products, whose molecular scaffold is quite difficult to reach by other synthetic approaches.
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