Journal
CRYSTENGCOMM
Volume 20, Issue 42, Pages 6721-6726Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8ce01287c
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Funding
- National Natural Science Foundation of China [21571090]
- Liaoning BaiQianWan Talents Program
- CINECA [2015XJA9NT_003]
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Nonporous hybrid metal-organic materials self-assembled by a ditopic organic ligand and copper(ii) have shown a dynamic behavior by releasing and trapping HCl. The solid-state process involves major structural reorganizations comprising cleavage and formation of coordination and covalent chemical bonds by mechanochemical reactions, heating reactions or chemisorption. Single crystal X-ray diffraction, powder X-ray diffraction and TGA in combination with DFT specific for solid-state systems have been used to study the solid-state reactivity.
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