Journal
CRYSTENGCOMM
Volume 15, Issue 20, Pages 4196-4200Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ce40213d
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Funding
- National Science Foundation of China [91022036, 11174297]
- National Key Fundamental Research (973) Program of China [2010CB630701]
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A new mixed halide, Hg2Br3I, has been synthesized in solution. It crystallizes in the noncentrosymmetric orthorhombic space group Cmc21 (no. 36). In its single crystal, the molecules are arranged in a shuttle-like mode. Its powders show a phase-matchable second harmonic generation (SHG) response of approximately 0.7 times as strong as that of KTiOPO4 (KTP). It also exhibits a wide transparent range (from 0.45 to 38 mu m) and a good thermal stability. These results indicate that Hg2Br3I is a promising candidate for NLO materials in the IR region.
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