Journal
CRYSTENGCOMM
Volume 14, Issue 10, Pages 3633-3637Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2ce06667j
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Funding
- National Research Foundation of Korea (NRF) [2011-0004065, 2010-0027743, 2011-0022978]
- Ministry of Education, Science and Technology
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We have designed and synthesized a new, highly efficient electro-optic vanillin-based quinolinium crystal. The HMQ-NS (2-(4-hydroxy-3-methoxystyryl)-1-methylquinolinium naphthalene-2-sulfonate) crystals exhibit an acentric monoclinic space group symmetry Pn with a large effective molecular hyperpolarizability in the crystal with the diagonal component beta(eff)(333) = 149 x 10(-30) esu, which is comparable to that of benchmark ionic stilbazolium crystals, and a good thermal stability. Therefore, the newly developed HMQ-NS crystal is an attractive candidate for nonlinear optical and electro-optic applications.
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