Journal
COMPTES RENDUS CHIMIE
Volume 11, Issue 8, Pages 818-833Publisher
ELSEVIER FRANCE-EDITIONS SCIENTIFIQUES MEDICALES ELSEVIER
DOI: 10.1016/j.crci.2008.04.003
Keywords
nickel-thiolates; iron-thiolate cyanocarbonyl; hydrogenases; model compound
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During the past decade, structures and functions (catalytic mechanism) of [NiFe]/[Fe] hydrogenases have been established/proposed. Model compounds, various biophysical measurements and theoretical calculations have been lent to elucidate the structure and function (catalytic mechanism) of active sites of [NiFe]/[Fe] hydrogenases. In this manuscript, biominetic model compounds, including iron(II)-thiolate cyanocarbonyls, nickel(III)-thiolates and nickel(II)-thiolate complexes with pendant thiol, are presented.
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