Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 54, Issue 19, Pages 5757-5761Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201501005
Keywords
batteries; green chemistry; electrochemical energy storage; electrode materials; nanomaterials
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Funding
- National Natural Science Foundation of China [51225204, 21303222, 21127901]
- National Basic Research Program of China [2011CB935700, 2012CB932900]
- Strategic Priority Research Program of the Chinese Academy of Sciences [XDA09010000]
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Rechargeable magnesium batteries have attracted recent research attention because of abundant raw materials and their relatively low-price and high-safety characteristics. However, the sluggish kinetics of the intercalated Mg2+ ions in the electrode materials originates from the high polarizing ability of the Mg2+ ion and hinders its electrochemical properties. Here we report a facile approach to improve the electro-chemical energy storage capability of the Li4Ti5O12 electrode in a Mg battery system by the synergy between Mg2+ and Li+ ions. By tuning the hybrid electrolyte of Mg2+ and Li+ ions, both the reversible capacity and the kinetic properties of large Li4Ti5O12 nanoparticles attain remarkable improvement.
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