Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 54, Issue 47, Pages 14066-14069Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201506432
Keywords
acyl radicals; acylarylation; carboxylic acids; oxindoles; photoredox catalysis
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Funding
- Olle Engkvist Byggmastare foundation
- Wilhelm and Martina Lundgren research foundation
- Ollie and Elof foundation
- Magnus Bergvall foundation
- Adlerbertska foundation
- Swedish Research Council
- European Commission [660668]
- Swedish NMR Centre at the University of Gothenburg
- Marie Curie Actions (MSCA) [660668] Funding Source: Marie Curie Actions (MSCA)
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Simple and abundant carboxylic acids have been used as acyl radical precursor by means of visible-light photoredox catalysis. By the transient generation of a reactive anhydride intermediate, this redox-neutral approach offers a mild and rapid entry to high-value heterocyclic compounds without the need of UV irradiation, high temperature, high CO pressure, tin reagents, or peroxides.
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