Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 54, Issue 31, Pages 9025-9028Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201503996
Keywords
gold; nanoframes; nanoparticles; platinum; surface plasmon resonance
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Funding
- Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy [DE-SC0010212]
- National Research Foundation of Korea (National Leading Research Lab) [NRF-2011-0027911]
- National Research Foundation of Korea (Pioneer Research Center) [2012-0009586]
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Herein, we report a general synthetic pathway to various shapes of three-dimensional (3D) gold nanoframes (NFs) embedded with a Pt skeleton for structural rigidity. The synthetic route comprises three steps: site-specific (edge and vertex) deposition of Pt, etching of inner Au, and regrowth of Au on the Pt framework. Site-specific reduction of Pt on Au nanoparticles (NPs) led to the high-quality of 3D Au NFs with good structural rigidity, which allowed the detailed characterization of the corresponding 3D metal NFs. The synthetic method described here will open new avenues toward many new kinds of 3D metal NFs.
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