Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 54, Issue 49, Pages 14875-14879Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201506990
Keywords
amination; C-H functinalization; cross-coupling; photoredox catalysis; synthetic methods
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Funding
- DST, New Delhi
- CSIR, New Delhi
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A conceptually new and synthetically valuable cross-dehydrogenative benzylic C(sp(3))-H amination reaction is reported by visible-light photoredox catalysis. This protocol employs DCA (9,10-dicyanoanthracene) as a visible-light-absorbing photoredox catalyst and an amide as the nitrogen source without the need of either a transition metal or an external oxidant.
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