Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 54, Issue 45, Pages 13297-13301Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201507058
Keywords
chemical stability; MOFs; phenolate; water adsorption; zirconium
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Funding
- labex CHARMMMAT [ANR-11-LABEX-0039]
- Region Ile-de France
- [ANR-12-JS08-0008]
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A novel Zr-chain based MOF, namely MIL-163, was designed and successfully synthesized using a bis-1,2,3-trioxobenzene ligand. Endowed with large square-shaped channels of 12 angstrom width, it shows remarkable water uptake (ca. 0.6cm(3)g(-1) at saturating vapor pressure) and a remarkable stability in simulated physiological media, where archetypical Zr carboxylate MOFs readily degrade.
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