Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 54, Issue 18, Pages 5451-5455Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201500067
Keywords
C-H functionalization; flow chemistry; metal catalysis; natural products; total synthesis
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Funding
- AstraZeneca
- Pfizer
- EPSRC
- ERC
- EPSRC [EP/I00548X/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [1127597, EP/I00548X/1] Funding Source: researchfish
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A sequential C-H functionalization strategy for the synthesis of the marine alkaloid dictyodendrin B is reported. Our synthesis begins from commercially available 4-bromoindole and involves six direct functionalizations around the heteroarene core as part of a gram-scale strategy towards the natural product.
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