Journal
CHINESE JOURNAL OF CHEMISTRY
Volume 31, Issue 4, Pages 479-484Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cjoc.201300094
Keywords
domino reaction; electron-deficient alkyne; acrylate; isatin; stereoselectivity
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Funding
- National Natural Science Foundation of China [21172189]
- Priority Academic Program Development of Jiangsu Higher Education Institutions
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The functionalized arylidene bis(3-arylaminoacrylates) were efficiently prepared by FeCl3 catalyzed one-pot domino reactions of primary amines, methyl propiolate and aromatic aldehydes. When isatins were utilized under similar conditions, only 2-oxoindolinyl 3-arylaminoacrylates were obtained in moderate yields. 1H NMR data and single crystal structures indicated that this reaction has high diastereoselectivity.
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