Journal
CHINESE JOURNAL OF CHEMICAL PHYSICS
Volume 26, Issue 3, Pages 310-320Publisher
CHINESE PHYSICAL SOC
DOI: 10.1063/1674-0068/26/03/310-320
Keywords
Dye-sensitized solar cell; Organic dye; Cobalt redox shuttle; Mass transport; Charge recombination
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Funding
- National Natural Science Foundation of China [21072152, 21101115]
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Developing photosensitizers suitable for the cobalt electrolyte and understanding the structure-property relationship of organic dyes is warranted for the dye-sensitized solar cells (DSSCs). The DSSCs incorporating tris (1,10-phenanthroline) cobalt (II/III)-based redox electrolyte and four synthesized organic dyes as photosensitizers are described. The photovoltaic performance of these dyes-sensitized solar cells employing the cobalt redox shuttle and the influences of the pi-conjugated spacers of organic dyes upon the photovoltage and photocurrent of mesoscopic titania solar cells are investigated. It is found that organic dyes with thiophene derivates as linkers are suitable for DSSCs employing cobalt electrolytes. DSSCs sensitized with the as-synthesized dyes in combination with the cobalt redox shuttle yield an overall power conversion efficiency of 6.1% under 100 mW/cm(2) AM1.5 G illumination.
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