Journal
CHIMIA
Volume 72, Issue 9, Pages 580-583Publisher
SWISS CHEMICAL SOC
DOI: 10.2533/chimia.2018.580
Keywords
Copper; Enantioselective synthesis; Eco-compatibility; Iron; Multi-catalysis; Organocatalysis
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Funding
- Agence Nationale pour la Recherche [ANR-13-PDOC-0007-01]
- Centre National de la Recherche Scientifique (CNRS)
- Aix-Marseille Universite
- Agence Nationale de la Recherche (ANR) [ANR-13-PDOC-0007] Funding Source: Agence Nationale de la Recherche (ANR)
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This article summarizes our recent developments in the discovery of multi-catalytic reactions. By efficiently taking the best from different worlds, the combination of several catalytic principles allows the invention of eco-compatible transformations rapidly assembling simple building blocks into elaborated enantioenriched molecules. This type of approach was successfully illustrated in the synthesis of cyclohexenones, keto-diols or in the direct functionalization of allylic alcohols by an enantioselective borrowing hydrogen. In addition, mechanistic understanding of the role of the different constituents enabled the fine-tuning of the catalytic systems considerably improving the efficiency notably in terms of enantiocontrol.
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