Journal
CHEMSUSCHEM
Volume 5, Issue 7, Pages 1313-1318Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cssc.201100466
Keywords
biomass; carbohydrates; heterogeneous catalysis; heteropolyacids; oxidation
Funding
- National Basic Research Program of China [2012CB215305, 2012CB215306]
- National Natural Science Foundation of China [21172209]
- Chinese Academy of Science [KJCX2-EW-J02]
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An efficient catalytic system for biomass oxidation to form formic acid was developed. The conversion of glucose to formic acid can reach up to 52?% yield within 3 h when catalyzed by 5 mol?% of H5PV2Mo10O40 at only 373 K using air as the oxidant. Furthermore, the heteropolyacid can be used as a bifunctional catalyst in the conversion of cellulose to formic acid (yield=35?%) with air as the oxidant.
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