Journal
CHEMPHYSCHEM
Volume 14, Issue 7, Pages 1387-1396Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cphc.201201094
Keywords
electron dynamics; lithium hydride; photoelectron spectroscopy; quantum wavepacket dynamics; time-resolved spectroscopy
Funding
- Ministry of Education, Culture, Sports, Science and Technology of Japan
- Grants-in-Aid for Scientific Research [23245002] Funding Source: KAKEN
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We theoretically study the application of a femtosecond pulse train to simultaneously probe the electronic excitation dynamics and nuclear vibrational motion in the excited-state LiH molecule by means of time-resolved photoelectron spectroscopy. The step-like population transfers caused by continual interaction with a sequence of pulses and refractory periods are shown to give rise to time evolution of the photoelectron kinetic energy distribution as the history of molecular electronic and vibrational states. Such a signal should lead to a novel and direct way to investigate electronic and nuclear simultaneous dynamics involving multiple excited states.
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