Journal
CHEMISTRY-AN ASIAN JOURNAL
Volume 13, Issue 20, Pages 2958-2977Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/asia.201801119
Keywords
annulation; bicyclization; radicals; reaction mechanisms; synthetic methods
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Funding
- NSFC [21602087]
- Priority Academic Program Development (PAPD) of Jiangsu Higher Education Institutions
- Outstanding Youth Fund of Jiangsu Normal University [YQ2015003]
- NSF of Jiangsu Province [BK20160212]
- Qing Lan Project of the Jiangsu Education Committee
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Over the past few years, the development of new radical reactions has gained considerable momentum. Most such radical transformations heavily depend on the insitu generation of reactive radical species, initiated by oxidants, metal salts, visible-light photocatalysis, or electrocatalysis. In this context, numerous radical-enabled bicyclization and annulation/1,n-bifunctionalization reactions have been developed, thereby providing efficient synthetic strategies for the assembly of functionalized cyclic rings that contain both heterocyclic and isocyclic skeletons. In this Focus Review, we highlight recent progress in this rapidly growing area by presenting a series of catalytic oxidative reactions, along with their reaction mechanisms and applications.
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