Journal
CHEMISTRY-AN ASIAN JOURNAL
Volume 10, Issue 1, Pages 112-115Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/asia.201402979
Keywords
asymmetric catalysis; CH; interaction; density functional calculations; hydrogenation; ruthenium
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Funding
- Grants-in-Aid for Scientific Research [13J04305] Funding Source: KAKEN
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The global reaction route mapping (GRRM) methods conveniently define transition states in asymmetric hydrogenation and transfer hydrogenation of aromatic ketones via the [RuH{(S,S)-TsNCH(C6H5)CH(C6H5)NH2}((6)-p-cymene)] intermediate. Multiple electrostatic CH/ interactions are the common motif in the preferred diastereometric structures.
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