Journal
CHEMISTRY-AN ASIAN JOURNAL
Volume 6, Issue 2, Pages 560-572Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/asia.201000544
Keywords
arynes; cross-coupling; cyclization; natural products; total synthesis
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Funding
- KAKENHI [20390003, 19890014, 21790006]
- Suntory Institute for Bioorganic Research
- Tohoku University
- JSPS
- Grants-in-Aid for Scientific Research [19890014, 21790006] Funding Source: KAKEN
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A highly efficient total synthesis of dictyodendrins A-E was accomplished. The synthesis features a novel benzyne-mediated one-pot indoline formation/cross-coupling sequence for the construction of a highly substituted key indoline intermediate. Peripheral substituents were introduced onto this intermediate in a modular fashion to complete the total synthesis of dictyodendrins A-E.
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