Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 24, Issue 67, Pages 17672-17676Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201804155
Keywords
colloidal tectonics; cyclodextrins; hybrid supramolecular structures; nanoparticles; polyoxometalates
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Funding
- Chevreul Institute [FR 2638]
- Ministere de l'Enseignement Superieur et de la Recherche
- Region Hauts-de-France
- Fonds Europeen de Developpement Regional (FEDER)
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Supramolecular hybrid functional nanoparticles (NPs) can be obtained via the colloidal tectonics approach provided that multiple interactive molecular tectons are used. Herein, the programmable synthesis of novel hybrid core-shell nanoparticles via the following sequential steps is reported: (i) complexation of 1-decanol by the beta-cyclodextrin (beta-CD), (ii) spontaneous self-assembly into CD NPs, (iii) adsorption of polyoxometalate anions, PW12O403-, on the polar neutral interface of the CD NPs. Such an approach paves the way for the design of novel and original materials and systems.
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