Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 24, Issue 59, Pages 15756-15760Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201803785
Keywords
enantiospecific; kinetics; larreatricin; polyphenol oxidase; total synthesis
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Funding
- Austrian Science Fund (FWF) [P29144]
- University of Vienna
- Austrian Science Fund (FWF) [P29144] Funding Source: Austrian Science Fund (FWF)
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A concise and efficient total synthesis of the lignan natural product larreatricin as well as an unambiguous assignment of configuration of its enantiomers are reported, resolving a long-held controversy. Enzyme kinetic studies revealed that different polyphenol oxidases show high and remarkably divergent enantioselective recognition of this secondary metabolite.
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