Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 24, Issue 69, Pages 18293-18306Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201803616
Keywords
hybrid materials; ionic conductivity; lithium metal anode; solid lithium batteries; solid-state electrolyte
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Funding
- China Postdoctoral Science Foundation [2018M632147]
- Thousand Young Talents Program of China
- Hundred Talents Program of Zhejiang University
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Conventional liquid electrolytes for lithium batteries usually suffer from irreversible decomposition and safety concerns. Solid state electrolytes (SSEs) have been considered as the key for advanced lithium batteries with improved energy density and safety, whereas challenges remain for polymer and inorganic SSEs. Recently, hybrid solid-state electrolytes (HSSEs) that integrate the merits of different electrolyte systems have been under intensive study. Herein, we summarize the recent progress of HSSEs with different compositions and structures. The design principle of each type of HSSEs are discussed, as well as their ionic conducting mechanism, electrochemical performance and effects of compositional/structural control. Finally, challenges and perspectives are provided for the future development of HSSEs and solid-state lithium batteries.
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