Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 21, Issue 5, Pages 1882-1887Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201405697
Keywords
CO2 hydrogenation; heterogeneous catalysis; hollow structures; manganese silicate; mesoporous materials
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Funding
- Ministry of Education, Singapore
- NUS
- GSK Singapore
- National Research Foundation (NRF), Prime Minister's Office, Singapore under its Campus for Research Excellence and Technological Enterprise (CREATE) program
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Manganese silicate in bubble-like morphology was used as a versatile platform to prepare a new class of yolk-shell hybrids. The mesoporosity of the shell was generated from the interbubble space and the bubble structure of manganese silica was used to hold and support nanoparticles (e.g., Au, Ag, Pt, Co, Ni, Au-Pd alloy, MoO2, Fe3O4, carbon nanotubes and their combinations). We also used heterogeneous catalysis reactions to demonstrate the workability of these catalysts in both liquid and gas phases.
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