Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 20, Issue 44, Pages 14189-14193Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201404462
Keywords
quinonlinone; carbonylation; CH activation; domino reactions; palladium
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Funding
- state of Mecklenburg-Vorpommern
- Deutsche Forschungsgemeinschaft
- Bundesministerium fur Bildung und Forschung (BMBF)
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We describe here a novel procedure for the synthesis of highly substituted 2-quinolinones. By this newly developed approach, 2-quinolinone derivatives were prepared in moderate to good yields by carbonylative cyclization of N-aryl-pyridine-2-amines and internal alkynes by CH activation. Remarkably, [Mo(CO)(6)] was applied as a solid CO source and the reaction proceeded in an atom economic manner.
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