Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 20, Issue 12, Pages 3258-3267Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201304586
Keywords
clusters; gas-phase chemistry; heterogeneous catalysis; mass spectrometry; reactivity
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Funding
- Stichting voor Fundamental Onderzoek der Materie (FOM)
- Max Planck Society
- Cluster of Excellence Unifying Concepts in Catalysis
- Deutsche Forschungsgemeinschaft (DFG)
- DFG [FI 893/3]
- Alexander von Humboldt Foundation
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Transition-metal clusters have long been proposed as model systems to study heterogeneous catalysts. In this Concept article we show how advanced spectroscopic techniques can be used to determine the structures of gas-phase transition-metal clusters and their complexes with small molecules. Combined with computational studies, this can help to develop an understanding of the reactivity of these catalytic models.
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