Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 18, Issue 51, Pages 16473-16477Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201203066
Keywords
amination; heterocycles; photocatalysts; redox chemistry
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Funding
- Funding Program for Next Generation World-Leading Researchers [GR025]
- MEXT, Japan
- JSPS
- Grants-in-Aid for Scientific Research [11J09130, 24105505] Funding Source: KAKEN
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Visible-light-mediated direct sp3 C?H amination of benzocyclic amines via a-aminoalkyl radicals by using photoredox catalysts is described here. The obtained N,N-acetals were also successfully applied for carboncarbon bond forming reactions with carbon nucleophiles. The procedure is suitable for a late-stage modification of C?H bonds to C?C bonds.
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