Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 16, Issue 31, Pages 9350-9365Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201001140
Keywords
asymmetric synthesis; Bronsted acids; combined catalysis; domino reactions; organocatalysis; transition metals
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Asymmetric catalysis is a key feature of modern synthetic organic chemistry. Traditionally, different combinations of ligands and metals are used to perform highly enantioselective reactions. Since the renaissance of organocatalysis in the early 2000s, tremendous improvement in the field of metal-free catalysis has been achieved. Recently, the combination of transition metals and organocatalysts has allowed the development of new protocols enabling transformations that could not previously be realized. This article aims to present the latest contributions in the field of combined chiral Bronsted acid and metal catalyzed reactions, highlighting the advantages of these catalytic systems as well as describing the uncertainties regarding the molecular structure of the catalytically active species and the reaction mechanisms.
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