Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 15, Issue 38, Pages 9632-9636Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.200901935
Keywords
allylic alkylation; C-H activation; homogeneous catalysis; palladium
Categories
Funding
- Danish National Research Foundation
- The Danish Council for Independent Research \ Technology and Production Sciences
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Recent breakthroughs have proved that direct palladium (II)-catalyzed allylic C-H alkylation can be achieved. This new procedure shows that the inherent requirement for a leaving group in the Tsuji-Trost palladium-catalyzed allylic alkylation can be lifted. These initial reports hold great promise for the development of allylic C-H alkylation into a widely applicable methodology, thus providing a means to enhance synthetic efficiency in these reactions.
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