Journal
CHEMISTRY OF MATERIALS
Volume 26, Issue 7, Pages 2438-2444Publisher
AMER CHEMICAL SOC
DOI: 10.1021/cm403921u
Keywords
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Funding
- State Key 973 Program of P. R China [2013CB934104, 2012CB224805]
- NSF of China [51372041, J1103304]
- Specialized Research Fund for the Doctoral Program of Higher Education of China [20120071110007]
- Innovation Program of Shanghai Municipal Education Commission [13ZZ004]
- Shanghai Rising Star Project of STCSM [12QH1400300]
- Shuguang Talents Program of Education Commission Shanghai [13SG02]
- Program for New Century Excellent Talents in University [NCET-12-0123]
- [RGP-227]
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Highly ordered mesoporous carbon/silica nanocomposites and dual-mesoporous silicas with a 3D cubic structure were successfully synthesized through a facile tricomponent coassembly approach by using the lab-made diblock copolymer poly(ethylene oxide)-b-polystyrene as a template. The mesoporous silicas exhibit a high surface area and uniform bimodal mesopores. The bimodal mesopores can be tuned by simply changing the ratio of carbon/silica precursors and the pyrolysis temperature in N-2. Gold nanoparticles were successfully loaded in the primary large mesopores for use as a heterogeneous nanacatalyst, which exhibits excellent performance in the epoxidation of styrene, demonstrating their potential for catalyst support.
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