Journal
CHEMISTRY LETTERS
Volume 42, Issue 6, Pages 654-656Publisher
CHEMICAL SOC JAPAN
DOI: 10.1246/cl.130133
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Funding
- JNC Petrochemical Corp.
- JNC Corp., JAPAN
- JSPS [23850010]
- Grants-in-Aid for Scientific Research [13J04935, 25810118, 25288091, 23850010] Funding Source: KAKEN
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We focus on aggregated structures and charge-transporting properties in semiconductor assemblies of a new-type twisted pi-conjugated molecule, dinaphtho[2,1-b:1',2'-d]furan (DNF-U). Single crystals were successfully grown by physical vapor transport to form a two-dimensional herringbone packing structure, which is advantageous for intermolecular charge transport. Based on the packing structure, relatively large transfer integrals were theoretically calculated to be 20 and 57 meV for C-H center dot center dot center dot pi and pi center dot center dot center dot pi direction, respectively. The single-crystal field-effect transistors exhibited notable hole mobility of up to 1.0 cm(2)V(-1)s(-1).
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