Journal
CHEMISTRY LETTERS
Volume 38, Issue 2, Pages 182-183Publisher
CHEMICAL SOC JAPAN
DOI: 10.1246/cl.2009.182
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Funding
- Grant-in-Aid for Scientific Research (A) [17205008]
- Grant-in-Aid for Specially Promoted Research [18002016]
- Grant-m-Aid for the Global COE Program
- Ministry of Education, Culture, Sports, Science and Technology of Japan.
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Experiments show that [Ru(terpy)(bpy)(OH2)](2+) is highly active as a catalyst toward oxidation of water into molecular oxygen in spite of the mononuclear character of the complex. while [Ru(terpy)(bpy)Cl](+) shows no activity at all. It is also confirmed that [Ru(terpy)(bpy)(OH2)](2+) is fairly stable under strongly oxidizing conditions in the presence of cerium(IV) ammonium nitrate, Ce(NH4)(2)(NO3)(6), which was evidenced by spectrophotometric, mass spectrometric, and gas chromatographic analysis.
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