Journal
CHEMICAL SOCIETY REVIEWS
Volume 47, Issue 19, Pages 7426-7451Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8cs00561c
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Funding
- German Research Foundation (DFG) within the Cluster of Excellence 'Center for Advancing Electronics Dresden' (cfaed)
- Initiative and Networking Fund of the German Helmholtz Association, Helmholtz International Research School for Nanoelectronic Networks NanoNet [VH-KO-606]
- Hamburg Science Award
- ERC
- National Natural Science Foundation of China [21720102002, 51722304]
- Shanghai Committee of Science and Technology [16JC1400703]
- Shanghai Pujiang Talent [18PJ1406100]
- EU Graphene Flagship
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Nowadays, the increasing requirements of portable, implantable, and wearable electronics have greatly stimulated the development of miniaturized energy storage devices (MESDs). Electrochemically active materials and microfabrication techniques are two indispensable parts in MESDs. Particularly, the architecture design of microelectrode arrays is beneficial to the accessibility of two-dimensional (2D) active materials. Therefore, this study reviews the recent advancements in microbatteries and microsupercapacitors based on electrochemically active 2D materials. Emerging microfabrication strategies enable the precise control over the thickness, homogeneity, structure, and dimension in miniaturized devices, which offer tremendous opportunities for achieving both high energy and power densities. Furthermore, smart functions and integrated systems are discussed in detail in light of the emergence of intelligent and interactive modes. Finally, future developments, opportunities, and urgent challenges related to 2D materials, device fabrications, smart responsive designs, and microdevice integrations are provided.
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