Journal
CHEMICAL SOCIETY REVIEWS
Volume 38, Issue 8, Pages 2169-2177Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/b815748k
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Funding
- National Science Foundation [CHE-0713880, CHE-0748738]
- American Chemical Society Petroleum Research Fund
- Division Of Chemistry [0748738] Funding Source: National Science Foundation
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Photoelectron imaging is finding increasingly widespread use in probing electronic structure and chemical dynamics. In this tutorial review, two benchmark systems, H(-) and I(-), are used to introduce essential concepts linking photoelectron images of negative ions with parent electronic structure. For pedagogical reasons, a qualitative approach based upon spectroscopic selection rules is emphasized in interpreting the images. This approach is extended to molecular systems, highlighting that even qualitative interpretation of results can lead to significant chemical insights.
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