Journal
CHEMICAL SOCIETY REVIEWS
Volume 37, Issue 4, Pages 623-638Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/b714577m
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Many of the active sites involved in electron transfer (ET) in biology have more than one metal and are mixed valent in at least one redox state. These include Cu-A, and the polynuclear Fe-S clusters which vary in their extent of delocalization. In this tutorial review the relative contributions to delocalization are evaluated using S K-edge X-ray absorption, magnetic circular dichroism and other spectroscopic methods. The role of intra-site delocalization in ET is considered.
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