Journal
CHEMICAL PHYSICS LETTERS
Volume 463, Issue 1-3, Pages 11-24Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.cplett.2008.08.059
Keywords
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Funding
- MURI program [FA9550-04-10242]
- US Department of Energy [DE-AC02-05CH11231]
- Alexander von Humboldt-Foundation
- National Science Foundation [CHE-072662]
- Direct For Mathematical & Physical Scien [0742662] Funding Source: National Science Foundation
- Division Of Chemistry [0742662] Funding Source: National Science Foundation
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The advent of attosecond pulsed radiation leads to a large unexplored scientific area in chemical physics: the direct time-resolved measurement of electronic quantum dynamics. Major scientific goals include spectroscopy of single- and multi-electron motion and dynamical electron correlations, relating to orbital interactions in valence and core electronic levels of atoms and molecules. The results of such studies address a wide array of scientific and technological applications. Here, the current state-of-the-art of attosecond-dynamics measurements is reviewed and several novel spectroscopic methods are discussed that are particularly important for applications in chemical physics: attosecond transient absorption/dispersion spectroscopy, laser-induced-dipole spectroscopy, and absolute-phase spectroscopy. (c) 2008 Elsevier B.V. All rights reserved.
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