Journal
CHEMICAL ENGINEERING SCIENCE
Volume 203, Issue -, Pages 511-525Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.ces.2018.09.012
Keywords
Circulating fluidized bed; Solar thermochemical cycles; DEM modeling; Particle-gas flow; Solar fuels
Categories
Funding
- Tenure Track Program, The Ministry of Education, Culture, and Sports, Science and Technology of Japan
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To perform thermochemical cycles using non-volatile metal oxides to split water and produce hydrogen, a directly irradiated fluidized bed reactor is designed and fabricated for beam-down configuration. As the main aim of this investigation is to analyze the heat transfer and particulate flow of the reactor, chemically inert particles are used. A transient 3D heat and mass transfer model is formulated by the combined approach of discrete element method and computational fluid dynamics. The radiative transfer is solved using the discrete ordinate radiation model. Experimental validation is accomplished by the measured temperatures, obtained with the fluidized bed reactor prototype tested under 30 kW(th) high-flux solar simulator. The model is applied to analyze the granular flow characteristics and efficiency of the reactor for various superficial gas velocities and bed masses. The results indicate that higher gas flow rate increases the velocity and convection loss of the bed and decreases the bed temperature and efficiency of the reactor. (C) 2018 Elsevier Ltd. All rights reserved.
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