4.6 Article

Experimental study on the effects of gas permeation through flat membranes on the hydrodynamics in membrane-assisted fluidized beds

Journal

CHEMICAL ENGINEERING SCIENCE
Volume 66, Issue 11, Pages 2398-2408

Publisher

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.ces.2011.02.059

Keywords

Chemical reactors; Fluidization; Membranes; Multi-phase flow; Particle Image Velocimetry; Hydrodynamics

Funding

  1. SenterNovem
  2. agency for sustainability and innovation within the Dutch Ministry of Economic Affairs

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Recently, many novel reactor concepts based on membrane fluidized bed reactors have been proposed. In this work, the effects of gas permeation through flat membranes on the hydrodynamics in a pseudo-2D membrane-assisted gas-solid fluidized bed have been investigated experimentally. A combination of the non-invasive techniques (Particle Image Velocimetry (PIV) and Digital Image Analysis (DIA)) was employed to simultaneously investigate solids phase and bubble phase properties in great detail. Counter-intuitively, addition of secondary gas via the membranes, that constituted the confining walls of a gas-solid suspension at conditions close to incipient fluidization, did not result in a larger, but in a smaller equivalent bubble diameter, while gas extraction on the other hand, resulted in a larger equivalent bubble diameter, although in this case the effect was less pronounced. This could be explained by changes in the larger scale particle circulation patterns due to gas extraction and addition via the membranes. (C) 2011 Elsevier Ltd. All rights reserved.

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