4.6 Article

Production of gas hydrate in a semi-batch spray reactor process as a means for separation of carbon dioxide from methane

Journal

CHEMICAL ENGINEERING RESEARCH & DESIGN
Volume 138, Issue -, Pages 168-175

Publisher

INST CHEMICAL ENGINEERS
DOI: 10.1016/j.cherd.2018.08.024

Keywords

Process; Gas hydrate; Spray reactor; Carbon dioxide; Separation

Funding

  1. ministry of science, technology and innovation of Malaysia under e-science project [06-02-02-SF0076]

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The formation of gas hydrate shows good potential to work as a separation medium for gas mixtures. However, to put it in practice, the impact of process parameters, such as flow rates, operational temperature and pressure are required to be adequately investigated. In this work, a new gas hydrate reactor is introduced for fast production of gas hydrate. The reactor is used for separation of carbon dioxide from methane in a series of semi-batch experiments. Results indicated that fast hydrate production is achievable. In addition, carbon dioxide is effectively separated from methane by producing gas hydrate from a gas mixture containing more than 60% carbon dioxide. (C) 2018 Institution of Chemical Engineers. Published by Elsevier B.V. All rights reserved.

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