Journal
CHEMICAL ENGINEERING JOURNAL
Volume 164, Issue 1, Pages 255-260Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2010.08.061
Keywords
Fe oxide; SBA-15; Advanced oxidation; Fenton reaction
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Mesoporous silica, SBA-15, supported Fe/SBA-15 catalysts were prepared by impregnation and tested for adsorption and heterogeneous advanced oxidation of 2,4-dichlorophenol (DCP) in aqueous solution using H2O2. Characterisation indicated that Fe impregnation did not change the porous structure of SBA-15. Fe/SBA-15 exhibits moderate DCP adsorption, however. Fe/SBA-15 is effective for DCP oxidation under H2O2. The catalytic activity depends on Fe loading, H2O2 concentration, DCP concentration and solution pH. Fe/SBA-15 can achieve 100% DCP conversion and 60% TOC removal at the conditions of 100 ppm DCP, 0.05g 10%wt Fe/SBA-15, and 1000 ppm H2O2. This catalyst also shows stable performance with low Fe leaching. (C) 2010 Elsevier BM. All rights reserved.
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